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Unloose (Verb)

Grant freedom to; free from confinement.

Verbs of political and social activities and events.

The governor decided to unloose the wrongly convicted prisoner from his lifelong sentence.
The police chief helped to unloose the hostages trapped in the building by negotiating with the kidnappers.
After the court's final verdict, the judge ordered to unloose the innocent man who had been held in jail for months.
The animal shelter decided to unloose the injured bird back into the wild after successful rehabilitation.
The government finally agreed to unloose the protesters who had been detained for peacefully expressing their opinions.

Loosen the ties of; "unloose your sneakers".

Verbs of touching, hitting, tying, digging.

Unloose your laces so I can tie them for you.
She had to unloose her tight grip on the steering wheel to shift gears smoothly.
Unloose the strings of your hoodie so I can see the logo on it.
The referee told the boxer to unloose his boxing gloves before the final round.
Be sure to unloose your grip on the rope before attempting to swing.